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Yuan, X.*; Hu, Q. H.*; Fang, X.*; Wang, Q. M.*; Ma, Y.*; Tachi, Yukio
Sedimentary Geology, 465, p.106633_1 - 106633_14, 2024/05
Zablackaite, G.; Shiotsu, Hiroyuki; Kido, Kentaro; Sugiyama, Tomoyuki
Nuclear Engineering and Technology, 56(2), p.536 - 545, 2024/02
Times Cited Count：0 Percentile：0.08(Nuclear Science & Technology)Fukuda, Kodai
Proceedings of 4th Reactor Physics Asia Conference (RPHA2023) (Internet), 4 Pages, 2023/10
Brief evaluations were performed using the N-F model to quantitatively clarify the effect of thermal expansion on the consequences of criticality accidents in the water-moderated fuel-particle-dispersion system. The analysis clarified that ignoring thermal expansion can lead to underestimation or overestimation of the consequences by several tens of percent. It is concluded that evaluators can ignore the thermal expansion when they evaluate the consequences of the prompt supercritical transient in water-moderated solid fuel-dispersion systems, such as fuel debris systems. Only the Doppler effect can be considered when the fuel-temperature-feedback coefficient is prepared. However, depending on the required accuracy, the evaluators should take care of the error caused by ignoring thermal expansion.
Nanjo, Kotaro; Shiotsu, Hiroyuki; Maruyama, Yu; Sugiyama, Tomoyuki; Okamoto, Koji*
Journal of Nuclear Science and Technology, 60(7), p.816 - 823, 2023/07
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)Vauchy, R.; Hirooka, Shun; Matsumoto, Taku; Kato, Masato
Frontiers in Nuclear Engineering (Internet), 1, p.1060218_1 - 1060218_18, 2022/12
Katano, Ryota; Yamamoto, Akio*; Endo, Tomohiro*
Nuclear Science and Engineering, 196(10), p.1194 - 1208, 2022/10
Times Cited Count：1 Percentile：29.26(Nuclear Science & Technology)In this study, we propose the ROM-Lasso method that enables efficient evaluation of sensitivity coefficients of neutronics parameters to cross-sections. In the proposed method, a vector of sensitivity coefficients is expanded by subspace bases, so-called Active Subspace (AS) based on the idea of Reduced Order Modeling (ROM). Then, the expansion coefficients are evaluated by the Lasso linear regression between cross-sections and neutronics parameters obtained by the random sampling. The proposed method can be applied in the case where the adjoint method is difficult to be applied since the proposed method uses only forward calculations. In addition, AS is an effective subspace that can expand the vector of sensitivity coefficients with the lower number of dimension. Thus, the number of unknows is reduced from the original number of input parameters and the calculation cost is dramatically improved compared to the Lasso regression without AS. In this paper, we conducted ADS burnup calculations as a verification. We have shown how AS bases are obtained and the applicability of the proposed method.
and GeO liquidsKawaguchi, Munemichi; Uno, Masayoshi*
Journal of Crystal Growth, 585, p.126590_1 - 126590_7, 2022/05
Phase-field mobility, 
, and crystal growth rates in crystallization of 11 oxides or mixed oxides in undercooled silicates, SiO and GeO liquids were calculated with a simple phase-field model (PFM), and material dependence of the was discussed. Ratios between experimental crystal growth rates and the PFM simulation with 
were confirmed to be proportional to a power of 
on the solid/liquid interface process during the crystal growth in a log-log plot. We determined that parameters, 
and 
, of the 
were 
to 
m
J
s and 
to 
, which were unique for the materials. It was confirmed that our PFM simulation with the determined reproduced quantitively the experimental crystal growth rates. The has a proportional relationship with the diffusion coefficient of a cation molar mass average per unit an oxygen molar mass at 
in a log-log graph. The depends on the sum of the cation molar mass per the oxygen molar mass, 
, in a compound. In 
, the decreases with the cation molar mass increasing. The assumed cause is that the B represents the degree of the temperature dependence of the . Since the cation molar mass is proportional to an inertial resistance of the cation transfer, the decreases with inverse of the cation molar mass. In crystallization of the silicates of heavy cation in 
, the saturates at approximately 0.67, which leads to 
.
Katano, Ryota; Yamamoto, Akio*; Endo, Tomohiro*
Proceedings of International Conference on Physics of Reactors 2022 (PHYSOR 2022) (Internet), p.2032 - 2041, 2022/05
We have proposed the ROM-Lasso method to perform an efficient evaluation of the sensitivity coefficients of ADS core parameters to cross sections without major modification of the core analysis system. In the ROM-Lasso method, the sensitivity coefficient vector is expanded via the subspace bases so-called Active Subspace (AS), and the effective number of unknowns is reduced. Then, the expansion coefficients are determined via the penalized linear regression with the core parameters obtained by the random sampling, and the sensitivity coefficient vector is estimated. Owing to the AS, the required number of the core calculations is dramatically reduced in the ROM-Lasso method. In this work, we take the sensitivity coefficient evaluation of the coolant void reactivity at the end of the cycle for example and demonstrate how estimation accuracy depends on the number of samples and the AS.
and Eu
ions onto sedimentary rock in the presence of gamma-irradiated humic acidZhao, Q.*; Saito, Takeshi*; Miyakawa, Kazuya; Sasamoto, Hiroshi; Kobayashi, Taishi*; Sasaki, Takayuki*
Journal of Hazardous Materials, 428, p.128211_1 - 128211_10, 2022/04
Times Cited Count：5 Percentile：59.24(Engineering, Environmental)The influence of humic acid and its radiological degradation on the sorption of Cs and Eu by sedimentary rock was investigated to understand the sorption process of metal ions and humic substances. Aldrich humic acid (HA) solution was irradiated with different doses of gamma irradiation using a Co-60 gamma-ray source prior to the contact between the metal ions and the solid sorbent. The HA molecule decomposed to smaller molecules with a lower complexation affinity. Batch sorption experiments were performed to evaluate the effect of gamma-irradiated HA on the sorption of Cs and Eu ions. The addition of non-irradiated HA weakened the sorption of Eu because of the lower sorption of the neutral or negatively charged Eu-HA complexes compared with free Eu ions. The sorption of monovalent Cs ions was barely affected by the presence of HA and its gamma irradiation. The concentration ratio of HA complexed species and non-complexed species in the solid and liquid phases was evaluated by sequential filtration and chemical equilibrium calculations. The ratios supported the minimal contribution of HA to Cs sorption. However, the concentration ratio for Eu in the liquid phase was high, indicating that the complexing ability of HA to Eu was higher than that of HA to Cs ions. Therefore, the sorption of free Eu would predominate with the gamma irradiation dose applied to the HA solution under a radiation field near the HLW package.
Hirooka, Shun; Yokoyama, Keisuke; Kato, Masato
Proceedings of International Conference on Fast Reactors and Related Fuel Cycles; Sustainable Clean Energy for the Future (FR22) (Internet), 8 Pages, 2022/04
Property studies on Am/Np-bearing MOX were carried out and how the properties influences on the irradiation behaviors was discussed. Both Am and Np inclusions increase the oxygen potential of MOX. Inter-diffusion coefficients obtained by using diffusion couple technique indicate that the inter-diffusion coefficient is larger in the order of U-Am, U-Pu and U-Np. Also, the inter-diffusion coefficients were evaluated to be larger at the O/M = 2 than those of O/M 
2 by several orders. The increase of oxygen potential with Am/Np leads to higher vapor pressure of UO
and the acceleration of the pore migration along temperature gradient during irradiation. The redistributions of actinide elements were also considered with the relationship of the pore migration and diffusion in solid state. Thus, the obtained inter-diffusion coefficients directly influence on the redistribution rate. The obtained properties were modelled and can be installed in a fuel irradiation simulation code.
-dispersed LATP by means of neutron radiographySong, F.*; Chen, H.*; Hayashida, Hirotoshi*; Kai, Tetsuya; Shinohara, Takenao; Yabutsuka, Takeshi*; Yao, Takeshi*; Takai, Shigeomi*
Solid State Ionics, 377, p.115873_1 - 115873_6, 2022/04
Times Cited Count：2 Percentile：28.85(Chemistry, Physical)Yokoyama, Kenji; Ishikawa, Makoto*
Annals of Nuclear Energy, 154, p.108100_1 - 108100_11, 2021/05
Times Cited Count：1 Percentile：15.7(Nuclear Science & Technology)In the design of innovative nuclear reactors such as fast reactors, the improvement of the prediction accuracies for neutronics properties is an important task. The nuclear data adjustment is a promising methodology for this issue. The idea of the nuclear data adjustment was first proposed in 1964. Toward its practical application, however, a great deal of study has been conducted over a long time. While it took about 10 years to establish the theoretical formulation, the research and development for its practical application has been conducted for more than half a century. Researches in this field are still active, and the fact suggests that the improvement of the prediction accuracies is indispensable for the development of new types of nuclear reactors. Massimo Salvatores, who passed away in March 2020, was one of the first proposers to develop the nuclear data adjustment technique, as well as one of the great contributors to its practical application. Reviewing his long-time works in this area is almost the same as reviewing the history of the nuclear data adjustment methodology. The authors intend that this review would suggest what should be done in the future toward the next development in this area. The present review consists of two parts: a) the establishment of the nuclear data adjustment methodology and b) the achievements related to practical applications. Furthermore, the former is divided into two aspects: the study on the nuclear data adjustment theory and the numerical solution for sensitivity coefficient that is requisite for the nuclear data adjustment. The latter is separated to three categories: the use of integral experimental data, the uncertainty quantification and design target accuracy evaluation, and the promotion of nuclear data covariance development.
Takahashi, Fumiaki; Manabe, Kentaro; Sato, Kaoru
JAEA-Review 2020-068, 114 Pages, 2021/03
JAEA-Review-2020-068.pdf:2.61MB
Radiation safety regulations have been currently established based on the 1990Recommendation by the International Commission on Radiological Protection (ICRP) in Japan. Meanwhile, ICRP released the 2007 Recommendation that replaces the 1990 Recommendation. Thus, the Radiation Council, which is established under the Nuclear Regulation Authority (NRA), has made discussions to incorporate the purpose of the 2007 Recommendation into Japanese regulations for radiation safety. As ICRP also has published effective dose coefficients for internal exposure assessment in accordance with the 2007recommendation, the technical standards are to be revised for the internal exposure assessment method in Japan. Currently, not all of the effective doses have been published to revise concentration limits for internal exposure protections of workers and public. The published effective dose coefficients are applied to radionuclides which are important in radiation protection for internal exposure of a worker. Thus, we review new effective dose coefficients as well as basic dosimetry models and data based upon Occupational Intakes of Radionuclides (OIR) parts 2, 3 and 4 that have been published from 2016 to 2019 by ICRP. In addition, issues are sorted out to provide information for revision of the technical standards for internal exposure assessment based on the 2007 Recommendations in future.
Yamaguchi, Tetsuji; Ohira, Saki; Hemmi, Ko; Barr, L.; Shimada, Asako; Maeda, Toshikatsu; Iida, Yoshihisa
Radiochimica Acta, 108(11), p.873 - 877, 2020/11
Times Cited Count：7 Percentile：65.65(Chemistry, Inorganic & Nuclear)Tachi, Yukio; Suyama, Tadahiro*; Mihara, Morihiro
JAEA-Data/Code 2019-021, 101 Pages, 2020/03
JAEA-Data-Code-2019-021.pdf:4.05MB
Sorption of radionuclides in cement and bentonite as engineered barrier materials, and rocks as natural barrier is the one of key processes in the performance assessment of geological disposal of TRU and high-level waste. The magnitude of sorption, expressed normally by a distribution coefficient (K
), needs to be measured and determined taking into account the properties of barrier materials and geochemical conditions and associated uncertainty in the performance assessment. The basic concept for TRU waste disposal contains cementitious materials as an engineered barrier materials, in addition to bentonite and rock. It is therefore needed to consider the effects of the cement degradation and co-existing substances such as nitrates on radionuclide sorption. This report focused on data acquisition of distribution coefficient (K) by batch sorption experiments for the systems coupling barrier material-chemical condition-radionuclides that are needed to consider for the performance assessment of geological disposal of TRU waste. The barrier materials considered are ordinary Portland cement (OPC), degraded OPC and tuff rock. The chemical conditions are distilled water and synthetic seawater equilibrated with OPC and those containing nitrates and ammonium salts, etc. The radionuclides considered are organic carbon, inorganic carbon, Cl, I, Cs, Ni, Se, Sr, Sn, Nb, Am and Th. Although K values have been partly reported previously as RAMDA (Radionuclide Migration Datasets) for the performance assessment in the TRU-2 report, these results and addition K data are reported with the details of experimental methods and conditions.
Sugino, Kazuteru; Numata, Kazuyuki*; Ishikawa, Makoto; Takeda, Toshikazu*
Annals of Nuclear Energy, 130, p.118 - 123, 2019/08
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)In MA sample irradiation test data calculations, the neutron fluence during irradiation period is generally scaled by using dosimetry data in order to improve calculation accuracy. In such a case, appropriate correction is required to burnup sensitivity coefficients obtained by the conventional generalized perturbation theory because some cancellations occur in the burnup sensitivity coefficients. Therefore, a new formula for the burnup sensitivity coefficient has been derived with the consideration of the neutron fluence scaling effect (NFS). In addition, the cross-section-induced uncertainty is evaluated by using the obtained burnup sensitivity coefficients and the covariance data based on the JENDL-4.0.
as a source of atmospheric I
Watanabe, Kosuke*; Matsuda, Shohei; Cuevas, C. A.*; Saiz-Lopez, A.*; Yabushita, Akihiro*; Nakano, Yukio*
ACS Earth and Space Chemistry (Internet), 3(4), p.669 - 679, 2019/04
Times Cited Count：8 Percentile：42.7(Chemistry, Multidisciplinary)The photooxidation of aqueous iodide ions (I
) at sea surface results in the emission of gaseous iodine molecules (I
) into the atmosphere. It plays a certain role in the transport of iodine from ocean to the atmosphere in the natural cycle of iodine. In this study, we determined the photooxidation parameters, the molar absorption coefficient (
(
)) and the photooxidative quantum yields (
()) of I, in the range of 290-500 nm. Through the investigation of the influence of pH and dissolved oxygen (DO) on (), the subsequent emission rates of I following the photooxidation of I in deionized water solution (pH 5.6, DO 7.8 mg L) and artificial seawater solution (pH 8.0, DO 7.0 mg L) were estimated. A global chemistry-climate model employed herein to assess the I ocean emission on a global scale indicated that the photooxidation of I by solar light can enhance the atmospheric iodine budget by up to 
8% over some oceanic regions.
Katano, Ryota; Endo, Tomohiro*; Yamamoto, Akio*; Tsujimoto, Kazufumi
Journal of Nuclear Science and Technology, 55(10), p.1099 - 1109, 2018/10
Times Cited Count：3 Percentile：29.78(Nuclear Science & Technology)In this study, we propose the penalized regression "adaptive smooth-lasso" for the estimation of sensitivity coefficients of the neutronics parameters. The proposed method estimates the sensitivity coefficients of the neutronics parameters using the variation of the microscopic cross sections and the neutronics parameter obtained by random sampling. The proposed method utilizes only the forward calculations. Thus, the proposed method can be applied for the complex reactor analysis for which the application of the adjoint method is difficult. In this study, we proposed a penalty term considering the characteristics of the sensitivity coefficients of the neutronics parameter to the microscopic multi-group cross sections. Through verification calculation, we show that the proposed method achieves high accuracy with less computational cost compared to the method based on random sampling proposed in the previous studies.
Dost
l, M.*; Rossiter, G.*; Dethioux, A.*; Zhang, J.*; Amaya, Masaki; Rozzia, D.*; Williamson, R.*; Kozlowski, T.*; Hill, I.*; Martin, J.-F.*
Proceedings of Annual Topical Meeting on Reactor Fuel Performance (TopFuel 2018) (Internet), 10 Pages, 2018/10
Wan, T.; Naoe, Takashi; Wakui, Takashi; Futakawa, Masatoshi; Obayashi, Hironari; Sasa, Toshinobu
Materials, 10(7), p.753_1 - 753_17, 2017/07
Times Cited Count：23 Percentile：72.44(Chemistry, Physical)